This paper presents the fourth extension to the Very Long Baseline Array (VLBA) Calibrator Survey, containing 258 new sources not previously observed with very long baseline interferometry (VLBI). This survey, based on three 24 hour VLBA observing sessions, fills remaining areas on the sky above declination -40 degr where the calibrator density is less than one source within a 4 degr radius disk at any given direction. The share of these area was reduced from 4.6% to 1.9%. Source positions were derived from astrometric analysis of group delays determined at 2.3 and 8.6 GHz frequency bands using the Calc/Solve software package. The VCS4 catalogue of source positions, plots of correlated flux density versus projected baseline length, contour plots and fits files of naturally weighted CLEAN images, as well as calibrated visibility function files are available on the Web at http://gemini.gsfc.nasa.gov/vcs4.